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Insights on atmospheric stratification and seasonal aerosol transport in North Pacific from trace metals in ice cores from the St. Elias Mountains, Yukon, Canada

Gross, Benjamin R H 1 ; Kreutz, Karl J 2 ; Osterberg, Erich 3 ; Handley, Mike 4 ; Sneed, Sharon 5

1 University of Maine Climate Change Institute
2 University of Maine Climate Change Institute
3 Dartmouth College
4 University of Maine Climate Change Inistitute
5 University of Maine Climate Change Institute

Mountainous regions around the world are sites of important atmospheric archives, yet heterogeneity of microclimates within individual alpine regions renders regional interpretation of these archives problematic. Analyzing a suite of similar archives that are spatially unique may help constrain the regional context under which archives from alpine regions interpreted. Chemical analyses of ice cores and snowpit samples from 3100 m.a.s.l. to 5300 m.a.s.l. in the St. Elias Mountains show evidence of regional atmospheric stratification. For example, the Pb flux from 1975 - 1998 as measured in ice cores from PR Col (5300 m.a.s.l.) and Eclipse Icefield (3100 m.a.s.l.) are statistically uncorrelated (R2 = 0.0468) suggesting that the sites are receiving distinct Pb inputs either by atmospheric stratification of Pb from a single source or by receiving Pb from different sources. Attempts to determine the source of these specific Pb aerosols are currently being undertaken using Pb isotope ratios (206Pb/208Pb and 207Pb/208Pb). Preliminary observations comparing Cs and U concentrations to the &deltaD timeseries for the Eclipse Icefield core possibly show seasonal signal related to the seasonality of trans-pacific transportation of continental dust.

Osterberg, E., P. Mayewski, K. Kreutz, D. Fischer, M. Handley, S. Sneed, C. Zdanowicz, J. Zheng, M. Demuth, M. Waskiewicz, J. Bourgeois, 2007, Ice core record of rising lead pollution in the North Pacific atmosphere: Geophysical Research Letters, In press.